Inorganic Substances as Additives in the Marine Aquarium



John W. Linville, D.V.M.



As an alternative to commercial trace element additives I would like to detail the possibility of making one's own solutions of the most common trace elements: calcium, strontium, iodine and bicarbonate.





Part II: The Cook Book

As far as making one's own solutions of the most common elements in the marine aquarium, I can only say it is a worthwhile effort. It does not take a genius or any special skills. One only needs an accurate scale, liquid measuring container and water. It is best to use distilled, or at the very least RO, water for this endeavor though.

Following are the "cook book recipes" for several elements. I will give general dosages for the elements, but remember that without accurately testing for them and just adding indiscriminately, a lot more harm can be done than good. Calcium, strontium, magnesium and bicarbonate all are in a balance with each other. In other words affecting the concentration of one will affect the concentration of the other. Indiscriminately adding one element without balancing it out with the other will wreak havoc on the system.

Also, I cannot take any responsibility for what might happen if you decide to make your own solutions. Chemical impurities, inexact weights and improper administration of the solutions can all cause disasters. But if you use good compounds, are tediously careful in the preparation, and administer, observe and test carefully, lots of satisfaction can be achieved by preparing one's own additives. Not to mention the savings that are possible compared to purchasing commercial products.

Where can the chemical substances be obtained? Local scientific warehouses and mail order companies are two possibilities. A search of the Internet will result in several companies specializing in these substances. Fisher Scientific, Aldrich, and Alfa Aesar are some of the better-known ones.





Calcium and Bicarbonate

Calcium: Ca; Ca2+ (ion); 40.08 (weight); 400 - 450 ppm (desired concentration)

Bicarbonate: HCO3- (ion); 61.0172 (weight)

The need for calcium in the marine aquarium is not in question. Hard corals utilize calcium in form of calcium carbonate in their skeletons. Soft corals, other invertebrates and fish need calcium for a number of biochemical processes.

What is in question these days is how to add the calcium. It can be added to the system in various forms and in several different ways. Adding Kalkwasser (Calcium Hydroxide -- Ca(OH)2) is an old and widespread method pioneered by Peter Wilkens. Opinions vary whether using Kalkwasser as the main source of calcium is prudent. A somewhat newer method of adding calcium is with calcium chloride (CaCl2) on its own. This method has the problem that when used alone, it creates an ionic imbalance by skewing the chloride ion concentration. The newest two-part additives compensate for this by adding sodium bicarbonate in balanced proportions. One can get around additives completely by using a kalk reactor. Personally I have had good luck with dripping Kalkwasser as my make up water (at night) and adjusting the calcium with calcium chloride.

Calcium (and strontium) is used in the form of its bicarbonate salt by marine organisms. These are then the ions that we naturally want to have available in our aquariums as the building blocks for this salt. This is a further advantage of the "two-part additives," as they raise the concentration of bicarbonate as well as calcium. Following is an illustration of how these additives work:

CaCl2 + 2NaHCO3 <==> Ca(HCO3)2 + 2NaCl

Or in other words, calcium chloride plus two (2) sodium bicarbonates react to calcium bicarbonate plus two (2) sodium chlorides. This reaction runs in both directions of course. It is evident though that by adding the compounds in this manner that the sodium and the chloride ions are balanced out. One only has to monitor the total salinity of the system and make adjustments accordingly. One also has to add other trace elements in their proportionate concentrations. This can be done with a good commercial trace element additive.

In Germany NaCl-free salts are also now available and can be used with this method. I am not aware of any NaCl-free salt for sale in the USA yet, but as interest in this method rises, I would say that it is only a matter of time before they can be purchased.

Martin Moe describes in his book, The Marine Aquarium Handbook, how to prepare a synthetic sea salt. If NaCl is left out of the mixture, a NaCl-free salt could be prepared. He calls for:

Sodium chloride 23.477g

Magnesium chloride 4.981g

Sodium sulfate 3.917g

Calcium chloride 1.102g

Potassium chloride 0.664g

Sodium bicarbonate 0.192g

Potassium bromide 0.096g

Boric acid 0.026g

Strontium chloride 0.024g

Sodium fluoride 0.003g

Commercial trace elements

This is the amount of salt normally used for 1 liter of water. Larger amounts would be needed. Multiplying the amounts by 100 or 1000 would make up sufficient salt mixture, and be easier to measure out as well.

Note: As can later be seen, the prepared solutions will not add twice as much sodium bicarbonate as calcium chloride. I can only surmise that Mr. Balling has good reasoning for this. One reason could be that chloride ions react with any number of other ions in the system. Another could be that too much bicarbonate will lower the pH over time. Bicarbonate is of course part of any good marine buffer, but lowers the pH to around 7.8 if not used in conjunction with borates and carbonates. Bicarbonates are also added in the third solution (NaCl-free salt solution) and must be accounted for.



To make the solutions:

(According to Hans Werner Balling)

375g of calcium chloride (anhydrous) is dissolved in 5000ml of water.

325g of sodium bicarbonate (baking soda) is dissolved in 5000ml of water.

150g of NaCl-free marine salt is dissolved in 5000ml of water.



These solutions are to be kept in separate containers and are stabile. If they were to be mixed, calcium carbonate would fall out and be useless in the aquarium.

Dosage: Initially add 30ml of each solution per 100 liters (approximately 25 gallons) of water, daily. Continue this until a carbonate hardness of 9 - 11 dH is reached. 30ml once or twice a week, per 100 liters should then suffice as a maintenance dose.

Carefully observe the animals and watch for any cramping. Test for calcium and adjust until a concentration of 400 - 450 ppm is achieved. While large pH swings are avoided with this method, testing is none the less essential. Large amounts of bicarbonate are added to the system but no borates or carbonates. A good commercial buffer will still be necessary to have on hand.



The CaCl2 solution is 0.68 molar (moles per liter).

The NaHCO3 solution is 0.77 molar.

1 mole of CaCl2 = 110.986g

1 mole of NaHCO3 = 84.007g



How can I accurately adjust my calcium level?

Determine the exact amount of water in the system. This is of course very difficult to do. Most people estimate how much water is in their system after adding rock, sand, etc. Subtract 10 - 30% of the total volume, depending on the amount of rock, etc. in the system. Do not forget to add the volume of water in the sump back in.

Determine the amount of calcium in the water. This is done with an accurate test kit.

Calculate how much calcium needs to be added to the system to reach the desired concentration.

Calculate how much calcium chloride solution this corresponds to.

Add equal amounts of all the solutions.



Example:

Our tank holds 55 gallons of water, has two inches of sand in the bottom, and rock pyramiding up the entire back wall. Furthermore the sump contains an additional 10 gallons of water. With the large amount of sand and rock, I would estimate that there is only about 70% of the volume in the tank as water. That turns out to be: 55 gallons x 70% = 38.5 gallons. Now we add the sump water volume to that and arrive at: 38.5 gallons + 10 gallons = 48.5 gallons. This is equivalent to 184.3l, or approximately 185 liters (1 gallon = 3.8 liters). Liters are easier to use in our calculations.

Our calcium test reads 360 ppm. We want 400ppm. This means we must increase our concentration by 40ppm. This is equivalent to 40mg/l or a one millimolar increase of the calcium concentration. Remember calcium weighs 40g per mole.

Our solution contains 375g of CaCl2 per 5000 ml. This equals 75g per 1000ml (1 liter). One mole of CaCl2 (anhydrous) weighs approximately 111g (110.986g to be exact). How many moles do we have per liter of our solution? 75g / 111g x 1 mole = 0.68 moles. Since there are 0.68 moles per liter, there are 680 millimoles (mM) per 1000ml or 0.68mM per ml.

We need a 1 millimolar (millimoles per liter) increase in Ca concentration. Our tank holds 185 liters of water, so we need 185 millimoles of Ca. Our solution contains 0.68mM of calcium per ml. We then need 185mM / 0.68mM x 1ml = 272ml of our solution. Equal amounts of all solutions are then added to the aquarium.

Note: When making such a large adjustment it is better to go slowly. This is what happens by following the 30ml daily routine. After the concentrations are where they should be, such large adjustments should no longer be necessary. 30ml once or twice a week, per 100 liters (approximately 25 gallons) of aquarium water should be ample as a maintenance dosage.



A similar example can be found on this web sight (Calculating how much Calcium to add, by Marty Boeckman)

This may seem complicated at first. After several computations it will become much easier. Remember though that we estimated several factors and rounded others. Again, I cannot stress enough, the importance of diligently testing the water conditions and observing the animals' reactions.

Note: Available calcium is also largely dependent on the amount of magnesium in the system. In other words, if the amount of available magnesium is depleted by say pink calcifying algaes, then the amount of available calcium will drop, due to the development of calcite. There is an extremely informative article on this on this web sight (Kalkwasser, Carbonate and Clumping, by Richard Greenfield).





Strontium

Strontium: Sr; Sr2- (ion); 87.62 (weight); 7-8 ppm (desired concentration)

Strontium is a necessary element for various corals (hard and leather corals). It performs vital functions in the uptake and use of calcium by these corals.

Care must be taken when dosing strontium. Erratic and too high doses of strontium (and also calcium for that matter) can lead to cramping of some smooth mushrooms (actinodiscus; smooth discosoma). In other words, regular dosing of smaller amounts is to be desired. It is also reported that strontium is only detectable for 36 hours after dosing. I have not tested this myself, but then I test my water several hours after dosing anyway.



To make the solution:

(According to Ernst Pawlowsky and Jürgen Thurau)

100g of SrCl2 (strontium chloride) are dissolved in 1000ml of water.



Dosage: Initially, 0.5ml of this 10% solution (weight / volume %) is used per 150 liters (approximately 40 gallons) of aquarium water, per week. Slowly increase the dosage to 1ml per 150 liters per week. This is the maximum recommended dosage.



A 10% SrCl2 solution is equivalent to a 0.63 molar (moles per liter) solution.

1 mole of SrCl2 = 158.526g





Iodine

Iodine: I (or J); I- (ion); 126.9045 (weight); 0.02-0.04 ppm (desired concentration)

Iodine is needed by various algaes, fish and shellfish. Iodine is also an important substance for the growth of mushrooms. Too much can lead to overgrowth of various algaes (especially bubble algae).



To make the solution:

(According to Fossa/Nilsen, modified by Jürgen Thurau)

100g of KI (potassium iodide) are dissolved in 1000ml of water (stock solution). This is a 10% (weight / weight %) solution.

10ml of the stock solution are added to 990ml of water to make a 10% additive solution. This is an example of a volume / volume percentage.



Dosage: 2.5ml per 100 liters (approximately 25 gallons) of aquarium water, per week.



The 10% stock solution is equivalent to a 0.60 molar solution.

The additive solution, which is 10% of the stock solution, is 0.06 molar.

1 mole of KI = 166.0065g





Final Notes:



Trace element solutions can be made for most any element. For the minute amounts of most other elements needed, commercial additives are the better solution.

Magnesium could easily be adjusted by making a magnesium chloride (MgCl2) solution. I do not have any data on such a solution at this. I also have not made this solution yet myself. I am planning on it in the near future though.

Nitrate can be added (?!?!?!) if necessary. Nitrates are needed by some brain corals and clams. By dissolving 1g of sodium nitrate (NaNO3) in 1000ml of water, a stock solution is prepared. At most 10ml of this solution are added per 100 liters (approximately 25 gallons) per week. Carefully watch this parameter if artificially adding nitrate please.

If any other commercial additives (e.g., Vital Gold or Combisan) are added, take the additional calcium, strontium and iodine into consideration. Homemade solutions may not be needed. At the very least less of the individual solutions will be necessary.



Sources and References:



Meernachrichten Marinlife, April 1997 (#25), Jürgen Thurau

Das Aquarium, # 315 & 317, Dieter Brockman and Alf Nielsen, Hans Werner Balling

Das Aquarium, # 301, Ernst Pawlowsky

Korallenriffaquarium, Band 1, Fossa/Nilsen

Riesenmuscheln, Daniel Knop

Albert Thiel's Web Sight, Albert Thiel, et al

The Marine Aquarium Handbook, Martin Moe



In the third and final installment, I will list some of the most common measures, conversions and some other useful data.

Part I: Inorganic Substances as Additives in the Marine Aquarium

Part III: of Inorganic Substances as Additives in the Marine Aquarium